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Polygodial: a viable natural product scaffold for the rapid synthesis of novel polycyclic pyrrole and pyrrolidine derivatives

Rihak, KJ, Bissember, AC ORCID: 0000-0001-5515-2878 and Smith, JA ORCID: 0000-0001-6313-3298 2018 , 'Polygodial: a viable natural product scaffold for the rapid synthesis of novel polycyclic pyrrole and pyrrolidine derivatives' , Tetrahedron, vol. 74, no. 12 , pp. 1167-1174 , doi: 10.1016/j.tet.2017.10.015.

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Abstract

The dialdehyde polygodial was utilised as a chiral scaffold for the unified synthesis of novel polycyclic pyrrole and pyrrolidine derivatives. Mechanistic insight into the reaction of primary amines with this dialdehyde was obtained. In addition, one of these polycyclic pyrroles was transformed further to prepare novel pentacyclic frameworks.

Item Type: Article
Authors/Creators:Rihak, KJ and Bissember, AC and Smith, JA
Keywords: polygodial, pyrrole, natural products, chiral synthetic scaffolds
Journal or Publication Title: Tetrahedron
Publisher: Pergamon-Elsevier Science Ltd
ISSN: 0040-4020
DOI / ID Number: 10.1016/j.tet.2017.10.015
Copyright Information:

Copyright 2017 Elsevier Ltd.

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